Place it at the end of a villain reveal or boast, then follow it with the Womp Womp Fail Sound when the plan collapses, or cut to JoJo To Be Continued to freeze the moment before the comeback. It also works as the payoff after a setup in a short anime edit.
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This is Gecko Moria's long, high-pitched kishishishi cackle from One Piece, lasting about ten seconds as it builds from amused chuckling into something more unhinged. It feels smug, eerie and theatrical, like a villain enjoying his own superiority a little too much. The former Warlord of the Sea and captain of the Thriller Bark Pirates, he uses it while letting his shadow-powered zombie crew do his fighting.